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NEB Calculations in vasp

Steps

GO for ini and fin structure

mind that IBRION = 2, and the atom index should be same.

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diff ini/POSCAR fin/POSCAR

relax INCAR

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Global Parameters
ISTART =  1            (Read existing wavefunction, if there)
ISPIN  =  1            (Non-Spin polarised DFT)
LREAL  = .FALSE.       (Projection operators: automatic)
ENCUT  =  600        (Cut-off energy for plane wave basis set, in eV)
LWAVE  = .False.        (Write WAVECAR or not)
LCHARG = .False.        (Write CHGCAR or not)
ADDGRID= .TRUE.        (Increase grid, helps GGA convergence)

Electronic Relaxation
ISMEAR =  0            (Gaussian smearing, metals:1)
SIGMA  =  0.05         (Smearing value in eV, metals:0.2)
NELM   =  90           (Max electronic SCF steps)
NELMIN =  6            (Min electronic SCF steps)
EDIFF  =  1E-05        (SCF energy convergence, in eV)
NCORE = 4

Ionic Relaxation
NSW    =  100          (Max ionic steps)
IBRION =  2            (Algorithm: 0-MD, 1-Quasi-New, 2-CG)
ISIF   =  2            (Stress/relaxation: 2-Ions, 3-Shape/Ions/V, 4-Shape/Ions)
EDIFFG = -2E-02        (Ionic convergence, eV/AA)

# Add VDW
IVDW = 11

for graphite, set IVDW = 11 vaspkit -task 102 -kps G -kpr 0

Check the ini and fin structure

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perl ./dist.pl ./ini/POSCAR ./fin/POSCAR

the structure should less than 5 A

Interpolate images

using the nebmake.pl script.

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perl nebmake.pl ./ini/CONTCAR ./fin/CONTCAR 1

Prepare INCAR for Standard Relax

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ISTART = 0
ICHARG = 2
ENCUT = 600
PREC = Medium
ISIF  = 2
LREAL = .FALSE.

ISMEAR = 0
SIGMA = 0.05
ISPIN = 2
NSW = 500
EDIFF = 1E-2
IBRION = 3
POTIM = 0
EDIFFG = -0.1

IOPT = 1
IVDW = 11
ICHAIN = 0
LCLIMB = .TRUE. 
IMAGES = 3 # the number set in nebmake
SPRING = -5

Sub calculation

check the convergence with nebef.pl

Results

use nebresults.pl to get the result

Reference

vasp做过渡态经验<一>

vasp-vtst计算过渡态(NEB方法)具体过程 - 知乎

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